Determination of the magnetic interactions of low-dimensional binary metal thiocyanates

Dr Matthew Cliffe, Dr Joseph Paddison, Mr Jeongjae Lee & Dr Tatiana Guidi
Magnetic molecular framework materials, where the magnetic metal centres are linked together by molecules rather than single atoms, are a very exciting class of materials, as they can combine the interesting features of molecular frameworks: porosity, flexibility and modularity with useful magnetic behaviour. Thiocyanate (NCS¿) is particularly interesting as a linker as it is unusually effective at transmitting magnetic coupling, but very little is known about the magnetic behaviour of the simple binary metal thiocyanates....
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